169 research outputs found
Spurious harmonic response of multipulse quantum sensing sequences
Multipulse sequences based on Carr-Purcell decoupling are frequently used for
narrow-band signal detection in single spin magnetometry. We have analyzed the
behavior of multipulse sensing sequences under real-world conditions, including
finite pulse durations and the presence of detunings. We find that these
non-idealities introduce harmonics to the filter function, allowing additional
frequencies to pass the filter. In particular, we find that the XY family of
sequences can generate signals at the 2fac, 4fac and 8fac harmonics and their
odd subharmonics, where fac is the ac signal frequency. Consideration of the
harmonic response is especially important for diamond-based nuclear spin
sensing where the NMR frequency is used to identify the nuclear spin species,
as it leads to ambiguities when several isotopes are present.Comment: 6 pages, 7 figure
Nuclear spin relaxation induced by a mechanical resonator
We report on measurements of the spin lifetime of nuclear spins strongly
coupled to a micromechanical cantilever as used in magnetic resonance force
microscopy. We find that the rotating-frame correlation time of the statistical
nuclear polarization is set by the magneto-mechanical noise originating from
the thermal motion of the cantilever. Evidence is based on the effect of three
parameters: (1) the magnetic field gradient (the coupling strength), (2) the
Rabi frequency of the spins (the transition energy), and (3) the temperature of
the low-frequency mechanical modes. Experimental results are compared to
relaxation rates calculated from the spectral density of the magneto-mechanical
noise.Comment: 4 pages, 4 figure
Feedback cooling of a cantilever's fundamental mode below 5 mK
We cool the fundamental mechanical mode of an ultrasoft silicon cantilever
from a base temperature of 2.2 K to 2.9 +/- 0.3 mK using active optomechanical
feedback. The lowest observed mode temperature is consistent with limits
determined by the properties of the cantilever and by the measurement noise.
For high feedback gain, the driven cantilever motion is found to suppress or
"squash" the optical interferometer intensity noise below the shot noise level.Comment: 4 pages, 6 figure
Force-detected nuclear double resonance between statistical spin polarizations
We demonstrate nuclear double resonance for nanometer-scale volumes of spins
where random fluctuations rather than Boltzmann polarization dominate. When the
Hartmann-Hahn condition is met in a cross-polarization experiment, flip-flops
occur between two species of spins and their fluctuations become coupled. We
use magnetic resonance force microscopy to measure this effect between 1H and
13C spins in 13C-enriched stearic acid. The development of a cross-polarization
technique for statistical ensembles adds an important tool for generating
chemical contrast in nanometer-scale magnetic resonance.Comment: 14 pages, 4 figure
An off-board quantum point contact as a sensitive detector of cantilever motion
Recent advances in the fabrication of microelectromechanical systems (MEMS)
and their evolution into nanoelectromechanical systems (NEMS) have allowed
researchers to measure extremely small forces, masses, and displacements. In
particular, researchers have developed position transducers with resolution
approaching the uncertainty limit set by quantum mechanics. The achievement of
such resolution has implications not only for the detection of quantum behavior
in mechanical systems, but also for a variety of other precision experiments
including the bounding of deviations from Newtonian gravity at short distances
and the measurement of single spins. Here we demonstrate the use of a quantum
point contact (QPC) as a sensitive displacement detector capable of sensing the
low-temperature thermal motion of a nearby micromechanical cantilever.
Advantages of this approach include versatility due to its off-board design,
compatibility with nanoscale oscillators, and, with further development, the
potential to achieve quantum limited displacement detection.Comment: 5 pages, 5 figure
Nuclear Magnetic Resonance Imaging with 90 nm Resolution
Magnetic resonance imaging, based on the manipulation and detection of
nuclear spins, is a powerful imaging technique that typically operates on the
scale of millimeters to microns. Using magnetic resonance force microscopy, we
have demonstrated that magnetic resonance imaging of nuclear spins can be
extended to a spatial resolution better than 100 nm. The two-dimensional
imaging of 19F nuclei was done on a patterned CaF2 test object, and was enabled
by a detection sensitivity of roughly 1200 nuclear spins. To achieve this
sensitivity, we developed high-moment magnetic tips that produced field
gradients up to 1.4x10^6 T/m, and implemented a measurement protocol based on
force-gradient detection of naturally occurring spin fluctuations. The
resulting detection volume of less than 650 zl represents 60,000x smaller
volume than previous NMR microscopy and demonstrates the feasibility of pushing
magnetic resonance imaging into the nanoscale regime.Comment: 24 pages, 5 figure
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